General Electric Research (GE) has partnered with the University of California, Berkeley (UCB) to develop an advanced integrated reticular sorbent-coated system to capture carbon dioxide (CO2) from the atmosphere ("AIR2CO2"). The system integrates pioneering metal-organic framework (MOF) sorbents and sorbent-binder composite coatings to capture and release atmospheric CO2. UCB is building on their benchmark MOF sorbent to synthesize, test, downselect, and sufficiently scale a next-generation sorbent with optimized overall CO2 adsorption capacity and thermal and chemical stability. GE is developing a robust MOF sorbent-binder formulation and coating process and integrating the advanced sorbent into an additively manufactured substrate. Component and system modeling of the AIR2CO2 process is being performed based on laboratory-scale experimental results and used to develop a techno-economic model that will inform future development of the sorbent material and AIR2CO2 contactor.